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                  [1]周毅,甘云華,楊澤亮.采用多元非線性回歸法的生物柴油動力學分析[J].哈爾濱工程大學學報,2020,41(7):1036-1042.[doi:10.11990/jheu.201902020]
                   ZHOU Yi,GAN Yunhua,YANG Zeliang.Kinetic analysis of biodiesel based on multivariate nonlinear regression method[J].hebgcdxxb,2020,41(7):1036-1042.[doi:10.11990/jheu.201902020]
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                  采用多元非線性回歸法的生物柴油動力學分析(/HTML)
                  分享到:

                  《哈爾濱工程大學學報》[ISSN:1006-6977/CN:61-1281/TN]

                  卷:
                  41
                  期數:
                  2020年7期
                  頁碼:
                  1036-1042
                  欄目:
                  出版日期:
                  2020-07-05

                  文章信息/Info

                  Title:
                  Kinetic analysis of biodiesel based on multivariate nonlinear regression method
                  作者:
                  周毅12 甘云華12 楊澤亮12
                  1. 華南理工大學 電力學院, 廣東 廣州 510640;
                  2. 廣東省能源高效清潔利用重點實驗室, 廣東 廣州 510640
                  Author(s):
                  ZHOU Yi12 GAN Yunhua12 YANG Zeliang12
                  1. School of Electric Power Engineering, South China University of Technology, Guangzhou 510640, China;
                  2. Guangdong Provincial Key Laboratory of Efficient and Clean Energy Utilization, Guangzhou 510640, China
                  關鍵詞:
                  生物柴油動力學熱解熱重分析動力學模型多元非線性回歸傅里葉紅外光譜升溫速率
                  分類號:
                  TK16
                  DOI:
                  10.11990/jheu.201902020
                  文獻標志碼:
                  A
                  摘要:
                  針對目前生物柴油的燃燒和熱解動力學分析不夠完善,本文采用熱重分析儀-傅里葉紅外變換光譜儀聯用對生物柴油分別進行氮氣和空氣氣氛下不同升溫速率的實驗,并分析所得到的熱重-熱失重速率(TG-DTG)曲線與紅外光譜圖。利用Kissinger法和Starink法分別計算出生物柴油在不同氣氛下的活化能與指前因子。以無模式函數法所求解的動力學參數作為初值,通過多元非線性回歸法求出相符的機理函數AG复古花园,并進行F-檢驗以驗證其回歸良好。結果表明:生物柴油熱解和燃燒熱重-熱失重速率的曲線變化規律一致,皆隨升溫速率的提高而向高溫區移動AG复古花园,且最大失重速率點接近;熱解和燃燒過程中氣態產物基本一致,僅在燃燒過程中在2 250~2 000 cm-1處檢測到一氧化碳的特征峰;多元非線性回歸法分析得出生物柴油熱解過程為單步動力學反應,燃燒過程為兩步連續動力學反應AG复古花园。實驗分析和回歸求出的機理函數,可用于生物柴油燃燒和熱解過程的化學反應動力學特性預測。

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                  備注/Memo

                  備注/Memo:
                  收稿日期:2019-02-22AG复古花园AG复古花园。
                  基金項目:國家自然科學基金項目(51776077);廣東省基礎與應用基礎研究基金項目(2020B1515020040);華南理工大學中央高;究蒲袠I務費資助項目(2018ZD05).
                  作者簡介:周毅,男,碩士研究生;甘云華,男,教授,博士生導師.
                  通訊作者:甘云華,E-mail:ganyh@scut.edu.cn.
                  更新日期/Last Update: 2020-08-15
                  AG复古花园

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